~ Soul Eater, it's a must. (Funny anime with lots of action and a good plot)
~ Shingeki no Kyojin, this anime will knock you off your feet. (Action, supernatural, it has giants eating humans who're fighting for survival and stunning plot twists)
~ Fullmetal Alchemist: Brotherhood (This anime has the best story/plot by far it's gut wrenching and it's full of action.)
And as Jingles said, Miyazaki has some amazing films. My favourite is Spirited Away.